Modeling and Simulation of Flexural Strength in Epoxy Graphene CNT Hybrids Using Python Tools

Main Article Content

Hatem Abdul Kareem Nori

Abstract

This paper provides a highly detailed experimental and predictive exploration of how to enhance flexural strength of polymer composites with the technique of bi-reinforced graphene nanoplatelets (GNP) and carbon nanotubes (CNT). One hundred and fifty hybrid combinations based on varying GNP (0-1 wt.%) and CNT (0-0.4 wt.%) contents were developed and prepared accordingly to determine the effects of hybrid fillers in flexural performance. Experimental findings showed that the un-reinforced baseline sample (0% GNP, 0% CNT) had flexural strength 68.90 MPa, whereas the strongest sample was recorded with 1% GNP and 0.3% CNT (120.20 MPa) which is an increment of 74.44 % as compared to the un-reinforced sample. Simultaneously, a regression model in the form of machine learning was trained to estimate the values of the flexural strength based on the filler contents as the input variables. The model proved very reliable with the highest strength being predicted as 100.85 MPa at the same optimum hybrid proportion, and lowest values of absolute and percent error in all specimens tested. The results of the model produced reasonably accurate results as compared to experimental data having R 2 values greater than 0.96, and an exclusively overlaying of predicted points on the 95 percent confidence interval.

Article Details

How to Cite
[1]
H. . Abdul Kareem Nori, “Modeling and Simulation of Flexural Strength in Epoxy Graphene CNT Hybrids Using Python Tools”, Rafidain J. Eng. Sci., vol. 3, no. 2, pp. 323–336, Sep. 2025, doi: 10.61268/7kwych97.
Section
Mechanical Engineering

How to Cite

[1]
H. . Abdul Kareem Nori, “Modeling and Simulation of Flexural Strength in Epoxy Graphene CNT Hybrids Using Python Tools”, Rafidain J. Eng. Sci., vol. 3, no. 2, pp. 323–336, Sep. 2025, doi: 10.61268/7kwych97.

References

Qin, Y., et al. (2020). Comparative study of CNT, GNP, and hybrid reinforcement in CFRP laminates. Carbon, 167, 511–522. https://doi.org/10.1016/j.carbon.2020.07.032

He, X., Zhang, Y., & Huang, Y. (2020). Mechanical properties of hybrid CNT-GNP epoxy nanocomposites under tensile loading. Applied Nanoscience, 10(9), 3021–3031. https://doi.org/10.1007/s42823-020-00161-x

Ahmed, A., & Ali, M. (2018). Experimental and numerical investigation of carbon-based hybrid cementitious composites. Magazine of Concrete Research, 71(8), 393–407. https://doi.org/10.1680/jmacr.18.00070

Rashid, R., et al. (2023). Advanced hybrid graphene and CNT ceramics for improved mechanical performance. Ceramics, 7(1), 112. https://doi.org/10.3390/ceramics7010112

Rasheed, A., et al. (2023). Hybrid GNP-CNT reinforcement in aluminum matrix composites. Materials Science and Engineering: A, 882, 145978. https://doi.org/10.1016/j.msea.2023.145978

Kamyab, H., et al. (2020). Hybrid nanofiller-reinforced fiber concrete: Mechanical and durability performance. Construction and Building Materials, 252, 119035. [PubMed ID: 26459823]

Jin, X., et al. (2020). Synergistic effects of CNT and GNP hybrid fillers in polymer composites. Materials Research Express, 7(1), 015601. https://doi.org/10.1088/2053-1591/ab5561

Abedi, M., et al. (2020). An effective method for hybrid CNT-GNP dispersion and its effects on mechanical properties of epoxy. Journal of Nanomaterials, 2020, Article ID 7690176. https://doi.org/10.1155/2020/7690176

Lu, D., et al. (2024). Nanofiller-modified cement pastes incorporating hybrid CNT-GNP. Discover Materials, 4(1), 1–12. https://doi.org/10.1007/s42114-024-01074-3

Wang, T., et al. (2025). Graphene and carbon nanotube reinforced composites fabricated via FDM for mechanical property improvement. Additive Manufacturing Letters, 6, 100173. https://doi.org/10.1016/j.amle.2025.100173

Abedi, H., Malekani, M., & Fereidoon, A. (2020). An effective method for hybrid CNT/GNP dispersion and its effects on the mechanical properties of epoxy nanocomposites. Journal of Nanomaterials, 2020, 1–11. https://doi.org/10.1155/2020/6657435

Basumatary, B. D., Debnath, B., & Debnath, K. (2021). The evaluation of flexural strength of coir, sisal and flax fiber composite. Materials Today: Proceedings, 47(1), 3132–3136. https://doi.org/10.1016/j.matpr.2021.04.567

Cheng, Q., Wang, B., & Zhang, Y. (2020). Strong and tough graphene oxide/polyimide nanocomposite film reinforced by amino-functionalized carbon nanotubes. Carbon, 170, 508–516. https://doi.org/10.1016/j.carbon.2020.07.032

Gurunathan, S., Han, J. W., Eppakayala, V., & Kim, J. H. (2019). Polymeric composites reinforced with graphene oxide: Physical, mechanical, and structural properties. Materials Research Express, 6(8), 085312. https://doi.org/10.1088/2053-1591/ab1cc2

Islam, M. S., Uddin, M. A., Rana, S., & Fangueiro, R. (2022). Graphene and CNT-based smart fiber-reinforced composites: A review. Advanced Functional Materials, 32(33), 2111972. https://doi.org/10.1002/adfm.202111972

Liu, Z., Zheng, S., Li, H., & Li, D. (2020). Enhancement of interlaminar fracture toughness and impact properties of carbon fiber/epoxy composites by CNT grown on carbon fiber surface. Journal of Applied Polymer Science, 137(41), 48828. https://doi.org/10.1002/app.48828

Qiu, H., Zhang, Z., & Gu, Y. (2015). Synergistic effects of hybrid carbon nanofillers on the mechanical and electrical properties of polypropylene composites. Carbon, 95, 228–238. https://doi.org/10.1016/j.carbon.2015.08.014

Tamer, A., Selmi, F., & Derbel, N. (2017). Effect of MWCNTs and GNPs hybrid nanofillers on the mechanical properties of epoxy resin. Materials Today: Proceedings, 5(1), 13968–13975. https://doi.org/10.1016/j.matpr.2017.12.243

Zakaria, M. N. A., Sapuan, S. M., Zuhri, M. Y. M., & Atiqah, A. (2021). Tensile and flexural strength of ramie fiber reinforced hybrid composites: Influence of fiber volume fraction. Journal of Natural Fibers, 18(12), 1574–1586. https://doi.org/10.1080/15440478.2019.1631529

Zhang, X., Li, Y., Wang, H., & Wu, J. (2019). Preparation of graphene/epoxy resin composites with enhanced mechanical and fracture properties. Advanced Functional Materials, 29(4), 1806822. https://doi.org/10.1002/adma.201908201

Abedi, H., Dehghan-Niri, E., & Nasouri, K. (2020). An effective method for hybrid CNT/GNP dispersion and its effects on the mechanical properties of epoxy-based nanocomposites. Journal of Nanomaterials, 2020, Article ID 4826458. https://doi.org/10.1155/2020/4826458

Islam, M. S., et al. (2022). Graphene and CNT-based smart fiber-reinforced composites: A review. Advanced Functional Materials, 32(20), 2200510. https://doi.org/10.1002/adfm.202200510

Gao, J., et al. (2015). The reinforcement of graphene oxide/carbon nanotubes on mechanical and thermal properties of epoxy composites. Carbon, 93, 742–749. https://doi.org/10.1016/j.carbon.2015.08.014

Qin, X., Zhang, D., & Wang, H. (2020). Synergistic reinforcement of epoxy coating with GNP and CNT on CFRP. Composites Part B: Engineering, 198, 108234. https://doi.org/10.1016/j.compositesb.2020.108234

Asmatulu, R., et al. (2014). Nanocomposite coatings for improved mechanical and corrosion protection. Materials & Design, 64, 111–117. https://doi.org/10.1016/j.matdes.2014.11.062

Kumar, A., et al. (2020). Experimental investigation on mechanical properties of GNP reinforced epoxy composite. Materials Today: Proceedings, 33, 1692–1696. https://doi.org/10.1016/j.matpr.2020.10.229

Wang, Y., et al. (2019). Improved interfacial properties and flexural performance in hybrid carbon–glass composites using carbon nanotubes. Composites Part B: Engineering, 175, 107539. https://doi.org/10.1016/j.compositesb.2019.107539

Edeerozey, A. M. M., et al. (2020). Tensile and flexural strength of ramie fiber reinforced epoxy composites with nanoclay. Materials, 16(5301), 1–11. https://doi.org/10.3390/ma16155301

Huang, Y., et al. (2019). Synergistic effects of GNPs and CNTs on enhancing mechanical and thermal properties of epoxy composites. Journal of Applied Polymer Science, 136(48), 34469. https://doi.org/10.1002/app.34469

Sui, G., et al. (2016). Enhanced crack resistance and fatigue behavior in epoxy nanocomposites reinforced with CNT/GNP hybrid fillers. Composites Part B: Engineering, 105, 44–52. https://doi.org/10.1016/j.compositesb.2016.05.035

Qin, J., Chen, X., Li, X., Zhang, L., & Wang, W. (2020). Effect of graphene nanoplatelets and carbon nanotubes on the flexural properties of carbon fiber reinforced epoxy composites. Composites Part B: Engineering, 200, 108288. https://doi.org/10.1016/j.compositesb.2020.108288